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澶嶅悎鏉愭枡
褰撳墠浣嶇疆錛?棣栭〉 >> 璧勮 >> 澶嶅悎鏉愭枡 >> 琛屼笟鍔ㄦ?/a> >> 姝ｆ枃

涓?/span>緙?/span>瑙?/span>鏃?/span>鐩?/span>绱?/span>寮?/span>鐨?/span>鑳?/span>婧?/span>闇姹?/span>鍜?/span>鐜?/span>澧?/span>姹?/span>鏌?/span>絳?/span>闂?/span>棰?/span>錛?/span>鍙?/span>灞?/span>鏂?/span>鍨?/span>鍙?/span>鍐?/span>鐢?/span>鑳?/span>婧?/span>鍔?/span>鍦?/span>蹇?/span>琛?/span>銆?/span>姘?/span>鑳?/span>浣?/span>涓?/span>涓縐?/span>鏂?/span>鍨?/span>娓?/span>媧?/span>鑳?/span>婧?/span>錛?/span>榪?/span>騫?/span>鏉?/span>宸?/span>緇?/span>寮?/span>璧?/span>浜?/span>瓚?/span>鏉?/span>瓚?/span>澶?/span>浜?/span>鐨?/span>鍏?/span>娉?/span>銆?/span>鍦?/span>鐜?/span>鏈?/span>鐨?/span>鍒?/span>姘?/span>鎶鏈?/span>涓?/span>錛?/span>鐢?/span>瑙?/span>姘?/span>鍒?/span>姘?/span>鍥?/span>鍏?/span>鏈?/span>鎿?/span>浣?/span>綆鍗?/span>銆?/span>姘?/span>綰?/span>搴?/span>楂?/span>鍜?/span>鍙?/span>鎸?/span>緇?/span>絳?/span>鐗?/span>鐐?/span>錛?/span>琚?/span>璁?/span>涓?/span>鏄?/span>鏈鍏?/span>鍓?/span>鏅?/span>鐨?/span>浜?/span>姘?/span>鎶鏈?/span>涔?/span>涓銆?/span>鐒?/span>鑰?/span>錛?/span>鍦?/span>鐢?/span>瑙?/span>姘?/span>鐨?/span>榪?/span>紼?/span>涓?/span>錛?/span>闃?/span>鏋?/span>鏋?/span>姘?/span>鍙?/span>搴?/span>錛?/span>HER錛?/span>緙?/span>鎱?/span>鐨?/span>鍔?/span>鍔?/span>瀛?/span>浠?/span>鍙?/span>浣?/span>鐨?/span>鑳?/span>閲?/span>杞?/span>鍖?/span>鐜?/span>錛?/span>鏋?/span>澶?/span>紼?/span>搴?/span>涓?/span>闄?/span>鍒?/span>浜?/span>璇?/span>鎶鏈?/span>鐨?/span>鍙?/span>灞?/span>銆?/span>鍥?/span>姝?/span>錛?/span>寮鍙?/span>鍏?/span>鏈?/span>楂?/span>鏁?/span>鏋?/span>姘?/span>鍙?/span>搴?/span>媧?/span>鎬?/span>涓?/span>鍦?/span>瀹?/span>pH鑼?/span>鍥?/span>鍐?/span>閫?/span>鐢?/span>鐨?/span>鐢?/span>鍌?/span>鍖?/span>鏉?/span>鏂?/span>鎴?/span>涓?/span>浜?/span>HER棰?/span>鍩?/span>鐨?/span>鐮?/span>絀?/span>鐑?/span>鐐?/span>鍜?/span>閲?/span>鐐?/span>銆?/span>


榪?/span>鏃?/span>錛?/span>杈?/span>瀹?/span>澶?/span>瀛?/span>鐔?/span>鑻?/span>鏁?/span>鎺?/span>銆?/span>鍚?/span>鏋?/span>澶?/span>瀛?/span>鏉?/span>鑻?/span>濞?/span>鏁?/span>鎺?/span>鍜?/span>姝?/span>姹?/span>縐?/span>鎶澶?/span>瀛?/span>姊?/span>宄?/span>鏁?/span>鎺?/span>鍥?/span>闃?/span>鍦?/span>鐢?/span>瑙?/span>姘?/span>鍒?/span>姘?/span>鏂?/span>闈?/span>鍙?/span>寰?/span>鏂?/span>榪?/span>灞?/span>錛?/span>璇?/span>欏?/span>宸?/span>浣?/span>浣?/span>鐢?/span>钁?/span>鑺?/span>鑴?/span>浣?/span>涓?/span>紕?/span>婧?/span>錛?/span>鎺?/span>絀?/span>浜?/span>瓚?/span>鍒?/span>瀛?/span>澶?/span>鐜?/span>鍖?/span>鍚?/span>鐗?/span>鍦?/span>姘?/span>鍒?/span>瑙?/span>鏂?/span>闈?/span>鐨?/span>搴?/span>鐢?/span>錛?/span>鐩?/span>鍏?/span>鎴?/span>鏋?/span>浠?/span>鏍?/span>棰?/span>涓?/span>鈥?/span>Iridium-Doped N-Rich Mesoporous Carbon Electrocatalyst with Synthetic Macrocycles as Carbon Source for Hydrogen Evolution Reaction鈥?/span>鍙?/span>琛?/span>鍦?/span>銆?/span>Advanced Functional Materials銆?/span>鏈?/span>鍒?/span>涓?/span>錛?/span>DOI:10.1002/adfm.202105562錛?/span>銆?/span>鏂?/span>绔?/span>絎?/span>涓浣?/span>鑰?/span>涓?/span>杈?/span>瀹?/span>澶?/span>瀛?/span>鍜?/span>鍚?/span>鏋?/span>澶?/span>瀛?/span>鑱?/span>鍩?/span>鍗?/span>澹?/span>鐢?/span>鑲?/span>嬈?/span>銆?/span>


鍥?/span>1 閾?/span>錛?/span>Ir錛?/span>瑁?/span>杞?/span>鐨?/span>钁?/span>鑺?/span>[6]鑴?/span>涓?/span>紕?/span>婧?/span>鐨?/span>鐢?/span>鍌?/span>鍖?/span>鍓?/span>CBC-Ir鐨?/span>鍚?/span>鎴?/span>紺?/span>鎰?/span>鍥?/span>銆?/span>


涓?/span>浼?/span>緇?/span>鐨?/span>紕?/span>婧?/span>鏉?/span>鏂?/span>濡?/span>鐭?/span>澧?/span>鐑?/span>銆?/span>紕?/span>綰?/span>綾?/span>綆?/span>銆?/span>MOFs鎴?/span>鍏?/span>浠?/span>綾?/span>鍨?/span>鐨?/span>紕?/span>婧?/span>鐩?/span>姣?/span>錛?/span>钁?/span>鑺?/span>鑴?/span>鑷?/span>韜?/span>鍏?/span>鏈?/span>鐙?/span>鐗?/span>鐨?/span>鑷?/span>緇?/span>瑁?/span>瀛?/span>緇?/span>鏋?/span>銆?/span>涓?/span>瀵?/span>鐨?/span>姘?/span>鎺?/span>鏉?/span>楠?/span>鏋?/span>浠?/span>鍙?/span>楂?/span>鐨?/span>閲?/span>灞?/span>紱?/span>瀛?/span>浜?/span>鍜?/span>鍔?/span>絳?/span>鐗?/span>鐐?/span>錛?/span>榪?/span>浜?/span>鐙?/span>鐗?/span>鐨?/span>鎬?/span>璐?/span>鑳?/span>澶?/span>鏈?/span>鏁?/span>鍦?/span>淇?/span>榪?/span>鐢?/span>瀛?/span>鐨?/span>浼?/span>杈?/span>銆?/span>鍥?/span>姝?/span>瓚?/span>鍒?/span>瀛?/span>鍚?/span>鎴?/span>澶?/span>鐜?/span>钁?/span>鑺?/span>鑴?/span>琚?/span>璁?/span>涓?/span>鏄?/span>涓縐?/span>鏋?/span>鏈?/span>鍓?/span>鏅?/span>鐨?/span>鍒?/span>澶?/span>楂?/span>鏁?/span>紕?/span>鍩?/span>鏉?/span>鏂?/span>鐨?/span>鍓?/span>椹?/span>浣?/span>銆?/span>璇?/span>欏?/span>宸?/span>浣?/span>浣?/span>鐢?/span>钁?/span>鑺?/span>鑴?/span>浣?/span>涓?/span>紕?/span>婧?/span>錛?/span>緇?/span>鍚?/span>璐?/span>閲?/span>灞?/span>閾?/span>錛?/span>Ir錛?/span>錛?/span>鏃?/span>闇娣?/span>鍔?/span>棰?/span>澶?/span>鐨?/span>姘?/span>婧?/span>鎴?/span>閫?/span>瀛?/span>妯?/span>鏉?/span>錛?/span>鍒?/span>澶?/span>浜?/span>涓緋?/span>鍒?/span>Ir綰?/span>綾?/span>綈?/span>瑁?/span>杞?/span>鐨?/span>姘?/span>鎺?/span>鏉?/span>鐨?/span>浠?/span>瀛?/span>紕?/span>鏉?/span>鏂?/span>錛?/span>CBC-Ir錛?/span>錛?/span>騫?/span>灝?/span>鍏?/span>搴?/span>鐢?/span>浜?/span>鐢?/span>瑙?/span>姘?/span>鍒?/span>姘?/span>銆?/span>寰?/span>鐩?/span>浜?/span>钁?/span>鑺?/span>鑴?/span>鐙?/span>鐗?/span>鐨?/span>瀛?/span>緇?/span>鏋?/span>浠?/span>鍙?/span>涓?/span>瀵?/span>鐨?/span>寮?/span>璐?/span>姘?/span>鎺?/span>鏉?/span>錛?/span>鎵鍒?/span>澶?/span>鐨?/span>鍌?/span>鍖?/span>鍓?/span>鑳?/span>澶?/span>鏆?/span>闇?/span>騫?/span>浜?/span>鐢?/span>鏇?/span>澶?/span>鐨?/span>HER媧?/span>鎬?/span>浣?/span>鐐?/span>錛?/span>鏈?/span>鏁?/span>鍦?/span>鎻?/span>楂?/span>浜?/span>鏉?/span>鏂?/span>鐨?/span>鍥?/span>鏈?/span>鍌?/span>鍖?/span>鎬?/span>鑳?/span>銆?/span>閫?/span>榪?/span>浼?/span>鍖?/span>鏉?/span>鏂?/span>鐨?/span>鍚?/span>鎴?/span>鏉?/span>浠?/span>濡?/span>鐓?/span>鐑?/span>娓?/span>搴?/span>錛?/span>800 鈩?/span>錛?/span>鍜?/span>閲?/span>灞?/span>閾?/span>鐨?/span>鍔?/span>鍏?/span>閲?/span>錛?/span>1.2 mg錛?/span>錛?/span>寰?/span>鍒?/span>鐨?/span>鏈浣?/span>鏉?/span>鏂?/span>CBC-Ir-800-1.2灞?/span>鐜?/span>鍑?/span>瓚?/span>楂?/span>鐨?/span>鐢?/span>鍌?/span>鍖?/span>媧?/span>鎬?/span>錛?/span>鍦?/span>0.5 M H2SO4鍜?/span>1.0 M KOH鐨?/span>鐢?/span>瑙?/span>璐?/span>鏉?/span>浠?/span>涓?/span>錛?/span>鐢?/span>嫻?/span>瀵?/span>搴?/span>涓?/span>10 mA cm-2鏃?/span>錛?/span>鍏?/span>榪?/span>鐢?/span>浣?/span>浠?/span>涓?/span>17鍜?/span>33 mV銆?/span>璇?/span>鍌?/span>鍖?/span>鎬?/span>鑳?/span>榪?/span>浼?/span>浜?/span>浣?/span>鐢?/span>鍏?/span>浠?/span>紕?/span>婧?/span>鎵鍒?/span>澶?/span>鐨?/span>鍌?/span>鍖?/span>鏉?/span>鏂?/span>濡?/span>CNT-Ir-800-1.2錛?/span>48.3/169.1 mV錛?/span>銆?/span>GO-Ir-800-1.2錛?/span>90.3/221.7 mV錛?/span>銆?/span>ZIF-Ir-900-1.2錛?/span>39.3/149.1 mV錛?/span>鐢?/span>鑷?/span>鏄?/span>鍟?/span>鐢?/span>Pt/C錛?/span>28/43 mV錛?/span>銆?/span>姝?/span>澶?/span>錛?/span>鏃?/span>璁?/span>鏄?/span>鍦?/span>0.5 M H2SO4榪?/span>鏄?/span>1.0 M KOH鐨?/span>鏉?/span>浠?/span>涓?/span>錛?/span>CBC-Ir-800-1.2鍧?/span>鍏?/span>鏈?/span>鑹?/span>濂?/span>鐨?/span>紼?/span>瀹?/span>鎬?/span>錛?/span>瓚?/span>楂?/span>鐨?/span>娉?/span>鎷?/span>絎?/span>浜?/span>姘?/span>鏁?/span>鐜?/span>錛?/span>91.5%鍜?/span>92.7%錛?/span>浠?/span>鍙?/span>浼?/span>寮?/span>鐨?/span>杞?/span>鎹?/span>棰?/span>鐜?/span>錛?/span>2.1鍜?/span>0.69 H2s?1錛?/span>銆?/span>


鍥?/span>2 鍦?/span>0.5 M H2SO4婧?/span>娑?/span>涓?/span>涓?/span>鍚?/span>紕?/span>婧?/span>鎵鍒?/span>澶?/span>鍌?/span>鍖?/span>鍓?/span>鐨?/span>鐢?/span>鍌?/span>鍖?/span>鎬?/span>鑳?/span>瀵?/span>姣?/span>錛?/span>錛?/span>a錛?/span>HER鏋?/span>鍖?/span>鏇?/span>綰?/span>錛?/span>錛?/span>b錛?/span>鏋?/span>鍖?/span>鏇?/span>綰?/span>鎵瀵?/span>搴?/span>鐨?/span>濉?/span>鑿?/span>灝?/span>鏂?/span>鐜?/span>錛?/span>錛?/span>c錛?/span>鍙?/span>鐢?/span>灞?/span>鐢?/span>瀹?/span>錛?/span>錛?/span>d錛?/span>鐢?/span>鍖?/span>瀛?/span>闃?/span>鎶?/span>錛?/span>錛?/span>e錛?/span>璐?/span>閲?/span>姣?/span>媧?/span>鎬?/span>浠?/span>鍙?/span>錛?/span>f錛?/span>娉?/span>鎷?/span>絎?/span>鏁?/span>鐜?/span>銆?/span>


鍥?/span>3 鍦?/span>1.0 M KOH婧?/span>娑?/span>涓?/span>涓?/span>鍚?/span>紕?/span>婧?/span>鎵鍒?/span>澶?/span>鍌?/span>鍖?/span>鍓?/span>鐨?/span>鐢?/span>鍌?/span>鍖?/span>鎬?/span>鑳?/span>瀵?/span>姣?/span>錛?/span>錛?/span>a錛?/span>HER鏋?/span>鍖?/span>鏇?/span>綰?/span>錛?/span>錛?/span>b錛?/span>鏋?/span>鍖?/span>鏇?/span>綰?/span>鎵瀵?/span>搴?/span>鐨?/span>濉?/span>鑿?/span>灝?/span>鏂?/span>鐜?/span>錛?/span>錛?/span>c錛?/span>鍙?/span>鐢?/span>灞?/span>鐢?/span>瀹?/span>錛?/span>錛?/span>d錛?/span>鐢?/span>鍖?/span>瀛?/span>闃?/span>鎶?/span>錛?/span>錛?/span>e錛?/span>璐?/span>閲?/span>姣?/span>媧?/span>鎬?/span>浠?/span>鍙?/span>錛?/span>f錛?/span>娉?/span>鎷?/span>絎?/span>鏁?/span>鐜?/span>銆?/span>


璇?/span>欏?/span>宸?/span>浣?/span>涓?/span>浠?/span>鎵?/span>灞?/span>浜?/span>瓚?/span>鍒?/span>瀛?/span>鍚?/span>鎴?/span>澶?/span>鐜?/span>鍦?/span>鐢?/span>鍌?/span>鍖?/span>姘?/span>鍒?/span>瑙?/span>鏂?/span>闈?/span>鐨?/span>搴?/span>鐢?/span>錛?/span>鑰?/span>涓?/span>涔?/span>涓?/span>鍚?/span>鐞?/span>璁?/span>璁?/span>鍜?/span>鐮?/span>鍙?/span>鍏?/span>鏈?/span>楂?/span>鍌?/span>鍖?/span>鎬?/span>鑳?/span>鐨?/span>紕?/span>鍩?/span>鐢?/span>鏋?/span>鏉?/span>鏂?/span>鎻?/span>渚?/span>浜?/span>鏂?/span>鐨?/span>鐮?/span>絀?/span>鎬?/span>璺?/span>銆?/span>


璇?/span>宸?/span>浣?/span>寰?/span>鍒?/span>浜?/span>鍥?/span>瀹?/span>鑷?/span>鐒?/span>縐?/span>瀛?/span>鍩?/span>閲?/span>錛?/span>21871108銆?/span>51674131鍜?/span>21373005錛?/span>銆?/span>鍚?/span>鏋?/span>鐪?/span>鐪?/span>鏍?/span>鍏?/span>寤?/span>欏?/span>鐩?/span>-鏂?/span>鏉?/span>鏂?/span>涓?/span>欏?/span>錛?/span>SXGJSF2017-3錛?/span>銆?/span>杈?/span>瀹?/span>鐪?/span>鑷?/span>鐒?/span>縐?/span>瀛?/span>鍩?/span>閲?/span>錛?/span>2019157錛?/span>銆?/span>鍥?/span>瀹?/span>縐?/span>鎶閮?/span>錛?/span>2015BAB02B03錛?/span>浠?/span>鍙?/span>杈?/span>瀹?/span>澶?/span>瀛?/span>鑷?/span>鐒?/span>縐?/span>瀛?/span>鍩?/span>閲?/span>錛?/span>LDGY2019009銆?/span>LDGY2019014錛?/span>鐨?/span>璧?/span>鍔?/span>銆?/span>


鐩?/strong>鍏?/strong>閾?/strong>鎺?/strong>

https://onlinelibrary.wiley.com/doi/10.1002/adfm.202105562

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